Just for the Record and not selling anything....Please check the first post and the guides we made there. This complete operation is a idiot-proof as changing a dying ATI card. Since we got OCLP working the rest is playing with a Lego set for children under six years, unless you can read.
You cannot sell an iMac with an macOS version without any support (High Sierra)! In less than a year you will face the first security aware websites not willing to connect to an older unsupported version of Safari, what will happen in 3 years when your ATI is dying, again?
We do not need to sell this solution to you. The market has already decided for you. GPU cards listed on post #1 became rare and expensive, no turnaround visible at the horizon.
If you love your old ATI so badly my personal advice:
Panta Rhei - „Denn alles muß in Nichts zerfallen, Wenn es im Sein beharren will“
Got two good working 6970m's lying around here just for that reason. if you want your system to be usable in the future there is no option but replacing them. Or stick with the outdated HS indeed.
Won't even sell them for exact you're own reason. Wouldn't like to have somebody coming back after 1-2 weeks that my overpriced card is also dying again.